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In general, medium-pore zeolites (ZSM-5 and ZSM-ll) are the best catalysts to produce hydrocarbons from methanol Below 300 C, the main reaction is dehydration of methanol to dimethyl ether With increasing temperature, however, the formation of hydrocarbons with a characteristic product distribution may be achieved The hydrocarbons formed are mainly C r C5 alkanes and C6-C IO aromatics with very little alkenes The aromatics are mostly methyl-substituted benzenes The much less than equilibrium concentration of tri- and tetramethyl-benzenes, and the sharp cutoff in product molecular weight, are attributed to zeolite shape selectivity The decrease in reactant partial pressure results in an increasing selectivity to alkenes Similarly, small-pore zeolites, which absorb linear hydrocarbons and exclude branched isomers, yield light hydrocarbons, mainly ethylene and propylene Increasing pressure, in contrast, leads to increasing aromatic substitution, giving durene (1 ,2,4,5-tetramethy lbenzene) with especially high selectivity.

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Important additional features of the medium-pore zeolite catalyzed process are the high octane number of the product formed and the excellent yields Medium-pore zeolites exhibit an exceptional resistance to coke deposition, ensuring long catalyst life More recently phosphorus-containing zeolites developed by Union Carbide (aluminophosphates, silicoaluminophosphates) were shown to be equally effective in methanol condensation 439-444 ZSM-5 was also shown to exhibit high activity and selectivity in the transformation of Fischer-Tropsch oxygenates to ethylene and propylene in high yields 445 Silicalite impregnated with transition-metal oxides, in turn, is selective in the production of C4 hydrocarbons (15-50% isobutane and 8-15% isobutylene)446 Bifunctional acid-based catalysts with no shape selectivity such as W0 3 on Al 20 3 have been found by Olah and coworkers to readily condense methanol or dimethyl ether (as well as monosubstituted methanes) to hydrocarbons.

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PDF417 - Wikipedia
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420,447 Primary products are ethylene and propylene, as well as light hydrocarbons, and methane and hydrogen The high yield of methane and hydrogen may be a consequence of some competing thermal reactions Hutchings and coworkers made further contributions concerning the mechanism 448 ,449 The mechanism of the conversion of methanol to hydrocarbons has been the subject of substantial studies 45 O--455 Despite the intensive research, however, many details of this very complex transformation remain unsolved It now appears generally accepted that methanol undergoes a preliminary Brpnsted acid-catalyzed dehydration step and that dimethyl ether, or an equilibrium mixture of dimethyl ether and methanol, acts as the precursor to hydrocarbon formation: 433.

The proximity of layout elements is one of the cues indicating relationships between them, so grouping elements is important. To achieve the desired effect, it s equally important to leave space between the groups of elements. In other words, the spaces you leave are as important as the elements you add, when it comes to the user interpreting the screen (or page) content. It s equally important to avoid clutter. If your table has many fields, consider showing only a manageable number of fields or groups of data on any one screen use multiple screens or multiple panels of a Tab Control to create separation between groups of fields. Aim to present the user with clear and striking ideas, allowing them to focus on the essential elements that are important at each step.

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